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Direct arylation of imidazo[1,2-a]pyridine at C-3 with aryl iodides, bromides, and triflates via copper(I)-catalyzed C-H bond functionalization.

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WOS被引频次:110
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成果类型:
期刊论文
作者:
Cao, Hua*;Zhan, Haiying;Lin, Yuanguang;Lin, Xiulian;Du, Zuodong;Jiang, Huanfeng
通讯作者:
Cao, Hua
作者机构:
[Jiang, Huanfeng] S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China.
[Lin, Yuanguang; Zhan, Haiying; Cao, Hua; Lin, Xiulian; Du, Zuodong] Guangdong Pharmaceut Univ, Sch Chem & Chem Engn, Guangzhou 510006, Guangdong, Peoples R China.
通讯机构:
[Cao, Hua] Guangdong Pharmaceut Univ, Sch Chem & Chem Engn, Guangzhou 510006, Guangdong, Peoples R China.
语种:
英文
期刊:
ORGANIC LETTERS
ISSN:
1523-7060
年:
2012
卷:
14
期:
7
页码:
1688-1691
文献类别:
WOS:Article
所属学科:
ESI学科类别:化学;WOS学科类别:Chemistry, Organic
入藏号:
WOS:000302387800008;PMID:22417233
基金类别:
Foundation for Distinguished Young Talentsin Higher Education of Guangdong, China [LYM11083]; National Natural Science Foundation of China [20932002, 21172076]; National Basic Research Program of China (973 Program) [2011CB808600]; Ministry of Education of China [20090172110014]; Guangdong Natural Science Foundation [10351064101000000]
机构署名:
本校为第一且通讯机构
院系归属:
医药化工学院
摘要:
A convenient method for the copper(I)-catalyzed arylation of substituted imidazo[1,2-a]pyridine has been developed. This method is applicable to a variety of aryl electrophiles, including bromides, iodides, and triflates. It represents the first general process for C-3 arylation of substituted imidazo[1,2-a]pyridine by Cu(I) catalysis to construct various functionalized imidazo[1,2-a]pyridine core pi-systems.
参考文献:
Ackermann L, 2006, ANGEW CHEM INT EDIT, V45, P2619, DOI 10.1002/anie.200504450
Ackermann L, 2005, ORG LETT, V7, P3123, DOI 10.1021/ol051216e
Ackermann L, 2008, ORG LETT, V10, P5043, DOI 10.1021/ol802252m
Ackermann L, 2010, TOP CURR CHEM, V292, P211, DOI 10.1007/128_2009_9
Alberico D, 2007, CHEM REV, V107, P174, DOI 10.1021/cr0509760

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